Dear Vladimir,
thank you for the excellent questions! As far as I understand, a carbon atom does not a priori have any magnetic moment. However, one can introduce magnetic moments by adding additional atoms of other elements "above" or "below" the carbon atoms; see for example this paper:
http://www.lnsm-zju.cn/lab/Upload/FCKfile/File/2008/5.pdf
Moreover, it seems that there is something like an emergent ferromagnetism going on, a phenomenon poorly understood. See here:
http://physicsworld.com/cws/article/news/19143
Finally, about extending the analysis to higher dimensions: Yes, I am indeed working on that! The goal is to see whether there are any higher-dimensional lattices which also have the property of the emergence of fermions. This is unlikely to be the case in 3D, since otherwise this would be well-known. I think that one would need a "non-rectangular" symmetry of the lattice. I'm not sure what exactly I mean by that, by the hexagonal graphene lattice certainly satisfies it with its ternary rotational symmetry, whereas an FCC lattice doesn't.
But I'm looking forward to study the 4D case, since this is the one relevant for actual physics in spacetime! (I'm thinking of things like lattice simulations of Euclidean Quantum Field Theory.)